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Verb: unloose  ,ún'loos
  1. Grant freedom to; free from confinement
    - free, liberate, release, unloosen, loose
     
  2. Loosen the ties of
    "unloose your sneakers";
    - unloosen

Derived forms: unlooses, unloosed, unloosing

Type of: unbrace, unlace, untie