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Verb: unloosen  ,ún'loo-sun
  1. Grant freedom to; free from confinement
    - free, liberate, release, unloose, loose
     
  2. Loosen the ties of
    "unloosen your sneakers";
    - unloose

Derived forms: unloosens, unloosening, unloosened

Type of: unbrace, unlace, untie